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So. There are some amazing artists who use spray paint as their primary medium. And one painter has made some fantastic glow-in-the-dark effects! For example, one of his Harry Potter pieces is so cool. (And about 11 minutes into his YouTube tutorial is where you can see the glow-y effect.)
My one disappointment with some of his work (besides the fact that they’re waaaay out of my price-range!) is that I’d love to see more of his backgrounds in natural daylight. For example, I love the background of his Sleeping Beauty piece. But you don’t really get to see it, except for some of the glow effects.